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You have an extra to in your sentence. I asked him not to do that.
edit: Section 4 addresses this basic grammar question:
Well....despite the "double preposition issue". I went to google Ngram viewer, and it really shows something:
- zero entries for "to not do" in any case
Tried present, past, him, her.....
On the other hand, I could not find any case of the subjunctive either, although I'm quite sure it's right (ask that he not do)
I have to agree with mark brosing here, "I asked him to not do that" is a perfectly valid sentence, if a little less common than "I asked him not to do that"
The link emeyr provides below this even confirms it, the general sentiment in that thread is "while 'asked him not to do that' is more common, 'asked him to not do that' is perfectly acceptable"
The rules that you "can't split infinitives" in english is a lot like the "you can't end a sentence in a preposition" rule, you absolutely can and it makes perfect sense (ex: where are you from? What was that about?) it's just that people decided a while back that they didn't like the way it sounds